Impact of hole transport material on perovskite solar cells with different metal electrode: A SCAPS-1D simulation insight
Электронный научный архив УРФУ
Информация об архиве | Просмотр оригинала| Поле | Значение | |
| Заглавие |
Impact of hole transport material on perovskite solar cells with different metal electrode: A SCAPS-1D simulation insight
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| Автор |
Danladi, E.
Gyuk, P. M. Tasie, N. N. Egbugha, A. C. Behera, D. Hossain, I. Bagudo, I. M. Madugu, M. L. Ikyumbur, J. T. |
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| Тематика |
DEFECT DENSITY
HTM METAL CONTACT PEROVSKITE SOLAR CELLS SCAPS-1D |
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| Описание |
The high efficiency and low cost of production of perovskite solar cells (PSCs) based on organic-inorganic halides have attracted the attention of researchers. However, due to the intricacy in the synthesis of Spiro-OMeTAD and the high cost of gold (Au) utilized as the back contact (BC), have affected its viability for commercialization. In this present study, a simulation was performed with and without HTM utilizing different metal contacts (Ag, Cr, Cu, Au, Ni and Pt). SCAPS-1D, a software program in one dimension, was used to conduct the simulation. A systematic analysis was done to determine how the metal back contact's work functions affected the PSC both with and without HTM. The outcomes demonstrate that the PSCs' photovoltaic performance is significantly influenced by the metal contact's work function (WF). The best metal contact for HTM and HTM-free devices was Pt, with a metal work function of 5.65 eV. The initial power conversion efficiencies (PCEs) for the two configurations were 26.229% for HTM-free and 25.608% for HTM-based device. A number of parameters, including absorber thickness, interface defect density, and electron transport material (ETM) thickness, were varied to obtain optimal values of 0.8 μm for both HTM and HTM-free PSCs, 1005 cm−2 for both HTM and HTM-free PSCs, and 0.01 μm for both HTM and HTM-free PSCs. These values were then used to simulate the final HTM and HTM-free devices with a PCE of 27.423%, current density (Jsc) of 27.546 mA/cm2, open circuit voltage (Voc) of 1.239 V, and fill factor (FF) of 80.347% for HTM-free whereas PCE of 26.767% with Jsc of 27.545 mA/cm2, Voc of 1.250 V, and FF of 77.733% for HTM based. These outcomes reflect outstanding enhancement of ∼1.05 and ∼1.07 times in PCE and Jsc over unoptimized cells with and without HTM. © 2023 The Authors
The SCAPS software package was created and made available for use by Professor Marc Burgelman and his team at the Department of Electronics and Information Systems at the University of Ghent in Belgium, for which the authors are grateful. |
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| Дата |
2024-04-05T16:25:13Z
2024-04-05T16:25:13Z 2023 |
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| Тип |
Article
Journal article (info:eu-repo/semantics/article) |info:eu-repo/semantics/publishedVersion |
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| Идентификатор |
Danladi, E, Gyuk, P, Tasie, N, Egbugha, A, Behera, D, Hossain, I, Bagudo, I, Madugu, ML & Ikyumbur, J 2023, 'Impact of hole transport material on perovskite solar cells with different metal electrode: A SCAPS-1D simulation insight', Heliyon, Том. 9, № 6, e16838. https://doi.org/10.1016/j.heliyon.2023.e16838
Danladi, E., Gyuk, P., Tasie, N., Egbugha, A., Behera, D., Hossain, I., Bagudo, I., Madugu, M. L., & Ikyumbur, J. (2023). Impact of hole transport material on perovskite solar cells with different metal electrode: A SCAPS-1D simulation insight. Heliyon, 9(6), [e16838]. https://doi.org/10.1016/j.heliyon.2023.e16838 2405-8440 Final All Open Access, Gold, Green https://www.scopus.com/inward/record.uri?eid=2-s2.0-85160605565&doi=10.1016%2fj.heliyon.2023.e16838&partnerID=40&md5=3202a3cd28bbd578394ae8d97b17dfd0 http://www.cell.com/article/S2405844023040458/pdf http://elar.urfu.ru/handle/10995/130532 10.1016/j.heliyon.2023.e16838 85160605565 001019341700001 |
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| Язык |
en
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| Права |
Open access (info:eu-repo/semantics/openAccess)
cc-by-nc-nd https://creativecommons.org/licenses/by-nc-nd/4.0/ |
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| Формат |
application/pdf
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| Издатель |
Elsevier Ltd
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| Источник |
Heliyon
Heliyon |
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