Computer simulation of thermal processes involving Sr and Ca radionuclides in the process of heating radioactive graphite in an air atmosphere
Электронный научный архив УРФУ
Информация об архиве | Просмотр оригиналаПоле | Значение | |
Заглавие |
Computer simulation of thermal processes involving Sr and Ca radionuclides in the process of heating radioactive graphite in an air atmosphere
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Автор |
Barbin, N. M.
Titov, S. A. Terentiev, D. I. Kobelev, A. M. |
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Тематика |
AIR ATMOSPHERE
EQUILIBRIUM CONSTANT HEATING RADIOACTIVE GRAPHITE RADIONUCLIDES THERMAL PROCESSES THERMODYNAMIC SIMULATION |
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Описание |
The paper presents the results from a thermodynamic analysis of the behavior of Sr and Ca radionuclides in the process of heating radioactive graphite in an air atmosphere. The TERRA software package was used for the thermodynamic analysis in a temperature range of 300 to 3600 K to determine the possible composition of the ionized, gaseous and condensed phases. It has been found that strontium is in the form of condensed SrCl2(c) and gaseous SrCl2 in a temperature range of 300 to 1600 K, and in the form of gaseous SrCl2, SrO, SrCl and Sr and ionized SrCl+, Sr+ and SrO+ when the temperature is increased from 1600 to 3600 K. Calcium is in the form of condensed CaCl2(c), CaUO4(c), CaO(c) and gaseous CaCl2 in the temperature interval between 300 and 2100 K, and in the form of gaseous Ca, CaCl and CaO and ionized Ca+, CaO+ and CaCl+ when the temperature is increased from 2100 to 3600 K. The paper determines the key reactions within individual phases and among condensed, gaseous and ionized phases. The equilibrium constants of their reactions have been calculated. Based on the results obtained, dependence plots are presented for the Sr and Ca radionuclide distribution by phases. © Barbin NM et al.
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Дата |
2024-04-05T16:38:55Z
2024-04-05T16:38:55Z 2023 |
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Тип |
Article
Journal article (info:eu-repo/semantics/article) |info:eu-repo/semantics/publishedVersion |
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Идентификатор |
Barbin, NM, Titov, SA, Terentiev, DI & Kobelev, AM 2023, 'Computer simulation of thermal processes involving Sr and Ca radionuclides in the process of heating radioactive graphite in an air atmosphere', Nuclear Energy and Technology, Том. 9, № 4, стр. 273-279. https://doi.org/10.3897/nucet.9.116661
Barbin, N. M., Titov, S. A., Terentiev, D. I., & Kobelev, A. M. (2023). Computer simulation of thermal processes involving Sr and Ca radionuclides in the process of heating radioactive graphite in an air atmosphere. Nuclear Energy and Technology, 9(4), 273-279. https://doi.org/10.3897/nucet.9.116661 2452-3038 Final All Open Access, Gold https://www.scopus.com/inward/record.uri?eid=2-s2.0-85181908857&doi=10.3897%2fnucet.9.116661&partnerID=40&md5=7b95f48ed1ddb62a1a84c6d47f0fb5e2 https://nucet.pensoft.net/article/116661/download/pdf/ http://elar.urfu.ru/handle/10995/131112 10.3897/nucet.9.116661 85181908857 |
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Язык |
en
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Права |
Open access (info:eu-repo/semantics/openAccess)
cc-by https://creativecommons.org/licenses/by/4.0/ |
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Формат |
application/pdf
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Издатель |
Pensoft Publishers
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Источник |
Nuclear Energy and Technology
Nuclear Energy and Technology |
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