The Stability of Hybrid Perovskites with UiO-66 Metal–Organic Framework Additives with Heat, Light, and Humidity
Электронный научный архив УРФУ
Информация об архиве | Просмотр оригинала| Поле | Значение | |
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The Stability of Hybrid Perovskites with UiO-66 Metal–Organic Framework Additives with Heat, Light, and Humidity
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| Автор |
Zhidkov, I. S.
Yu, M. -H. Kukharenko, A. I. Han, P. -C. Cholakh, S. O. Yu, W. -Y. Wu, K. C. W. Chueh, C. -C. Kurmaev, E. Z. |
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| Тематика |
HYBRID PEROVSKITES
METAL–ORGANIC FRAMEWORKS STABILITY UIO-66 XPS |
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| Описание |
This study is devoted to investigating the stability of metal–organic framework (MOF)-hybrid perovskites consisting of CH3NH3PbI3 (MAPbI3) and UiO-66 without a functional group and UiO-66 with different COOH, NH2,and F functional groups under external influences including heat, light, and humidity. By conducting crystallinity, optical, and X-ray photoelectron spectra (XPS) measurements after long-term aging, all of the prepared MAPbI3@UiO-66 nanocomposites (with pristine UiO-66 or UiO-66 with additional functional groups) were stable to light soaking and a relative humidity (RH) of 50%. Moreover, the UiO-66 and UiO-66-(F)4 hybrid perovskite films possessed a higher heat tolerance than the other two UiO-66 with the additional functional groups of NH2 and COOH. Tthe MAPbI3@UiO-66-(F)4 delivered the highest stability and improved optical properties after aging. This study provides a deeper understanding of the impact of the structure of hybrid MOFs on the stability of the composite films. © 2022 by the authors.
Russian Foundation for Basic Research, РФФИ, (21-52-52002) Ministry of Education, MOE, (109M4074, 111L9006) Ministry of Education and Science of the Russian Federation, Minobrnauka National Taiwan University, NTU, (111L7818) National Science and Technology Council, NSTC, (109-2628-E-002-008-MY3, 110-2923-E-002-007-MY3, 111-2124-M-002-021, 111-2628-E-002-009, 111-2634-F-002-016, 111-2923-E-002-006-MY3) The XPS measurements were supported by Russian Foundation for Basic Research (projects No. 21-52-52002). I.S.Z. and A.I.K gratefully acknowledge the funding from the Ministry of Science and Higher Education of the Russian Federation (Ural Federal University Program of Development within the Priority-2030 Program). C.-C.C. is grateful for the financial support from the National Science and Technology Council (NSTC) in Taiwan (111-2634-F-002-016, 109-2628-E-002-008-MY3, 110-2923-E-002-007-MY3, 111-2923-E-002-006-MY3, 111-2628-E-002-009, 111-2124-M-002-021), the Top University Project of National Taiwan University (111L7818), and the Ministry of Education (MOE) in Taiwan (109M4074 and 111L9006). |
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| Дата |
2024-04-08T11:06:50Z
2024-04-08T11:06:50Z 2022 |
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| Тип |
Article
Journal article (info:eu-repo/semantics/article) Published version (info:eu-repo/semantics/publishedVersion) |
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| Идентификатор |
Zhidkov, IS, Yu, MH, Kukharenko, AI, Han, PC, Cholakh, SO, Yu, WY, Wu, KCW, Chueh, CC & Kurmaev, EZ 2022, 'The Stability of Hybrid Perovskites with UiO-66 Metal–Organic Framework Additives with Heat, Light, and Humidity', Nanomaterials, Том. 12, № 23, 4349. https://doi.org/10.3390/nano12234349
Zhidkov, I. S., Yu, M. H., Kukharenko, A. I., Han, P. C., Cholakh, S. O., Yu, W. Y., Wu, K. C. W., Chueh, C. C., & Kurmaev, E. Z. (2022). The Stability of Hybrid Perovskites with UiO-66 Metal–Organic Framework Additives with Heat, Light, and Humidity. Nanomaterials, 12(23), [4349]. https://doi.org/10.3390/nano12234349 2079-4991 Final All Open Access; Gold Open Access; Green Open Access https://www.mdpi.com/2079-4991/12/23/4349/pdf?version=1670564850 https://www.mdpi.com/2079-4991/12/23/4349/pdf?version=1670564850 http://elar.urfu.ru/handle/10995/131354 10.3390/nano12234349 85143663380 000897566300001 |
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| Язык |
en
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| Права |
Open access (info:eu-repo/semantics/openAccess)
cc-by https://creativecommons.org/licenses/by/4.0/ |
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| Формат |
application/pdf
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| Издатель |
MDPI
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| Источник |
Nanomaterials
Nanomaterials |
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